Dissertation of bcps

Dissertation of bcps

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"Morphology and Properties of Styrene-Based Block Copolymers (BCPS) and" by Tety Kwee

A Showcase of scholarship, research, and creativity at the university of southern mississippi. Tety Kwee. Due to the ability of block copolymers BCPs to dissertation of bcps and form microphase separated morphologies, a great deal of interest has been focused on developing unique materials utilizing this self-assembly behavior.

Several types of BCPs are used as morphological template to create these nanocomposites. In addition, various architectures of BCPs based on polyisobutylene PIB middle block and PS outer blocks were also used in this regard, dissertation of bcps. The morphologies of these BCPs were evaluated prior to nanocomposite fabrication. The unmodified mSEBS, assumed hexagonally packed PS cylinders HPCand this morphology remained unperturbed at low sulfonation levels, dissertation of bcps.

As the sulfonation level increases, these PS cylinders become 'frustrated' implying that there are chain associations in the form of hydrogen bonding within the sulfonate groups. The sulfonated mSEBS smSEBS morphologies become further 'frustrated' upon inclusion of the silicate phase, suggesting that the formation of the silicate quasi-network impedes the kinetic mobility of the sulfonated PS sPS chains during film formation, consequently disrupting the long-range equilibrium microstructures.

The types of silicate monomers and BCP architecture also influence the size, shape, and distributions of the silicate particles, dissertation of bcps. Large and non-uniform silicate particles were seen in the nanocomposites derived from semi-organic monomers with large pendant groups. Similarly, the silicate structures also became increasingly irregular with increasing number of arms in BCPs. These results suggest that there is an inherent competition between the diffusion rate of the silicate monomers and BCP film formation, dissertation of bcps.

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Privacy Copyright. Skip to main content. Home About FAQ My Account. Author Tety Kwee. Department Polymers and High Performance Materials. Advisor Department Polymers and High Performance Materials. Abstract Due to the ability of block copolymers BCPs to self-assemble and form microphase separated morphologies, a great deal of dissertation of bcps has been focused on developing unique materials utilizing this self-assembly behavior.

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